You should definitely give 'Still Life' a go. Dark and serious atmosphere and the music and sound effects really add to the experience.
One of the best stories that can be found in an adventure game, at least if you ask me.
Other good choices would be these:
Overclocked: A history of violence
Post Mortem (Prequel to Still Life, but not as good imho)
Alter Ego
Sinking Island
Syberia 1 & 2
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