Rolf Saxon as George Stobbart definitely, in fact the entire cast of Broken Sword 1, 2 & 3. Dominic Armato as Guybrush Threepwood including the rest of the cast for CofMI, the guy who plays Lewton in Discworld Noir, Eric Idle as Rincewind, Tim Curry in Gabriel Knight 1 (his voice acting in 3 sounded a tad over the top compared to the first), Mark Hamill as Mosely. I'd also agree that the voice acting in the LucasArts games are excellent, even though the guy who does the voice of Marcus Brody in FoA was laughable. 
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Now Playing: Broken Sword: Shadow of the Templars - The Director's Cut (DS and iPhone), DOOM 3: Resurrection of Evil, Hotel Dusk: Room 215, Phoenix Wright: Ace Attorney Justice for All, Silent Hill - HD Collection
Recently Completed: Max Payne, Max Payne 2: The Fall of Max Payne
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