The Dig - in terms of atmosphere this is number 1 for me
Anachronox - I agree with Winterfury, and the game is simply stunning
Dreamweb - raining, dreaming, killing
Pandora Directive - the unique post-apocalyptic/noir world
Gateway 2 - truly original settings and one of the best book adaptations
I also hope to play Omikron and Outcast some day - even the demos were dripping with atmosphere.
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