I like most OST for
Dune - best soundtrack from Cryo, and that means best soundtrack for a adventure game
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Spice Opera
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Chanis Eyes
Apart from Dune, I also like OST from Outcast, QFG IV, Gabriel Knight 2, Machinarium, The Dig, Fallout and The Neverhood.
And a few memorable ones:
Mr. Handagote - Machinarium
Assassins Creed II OST - Flight Over Venice 1
12. Angela - Gray Matter
Outlaws - The Last Gunfight
